Article information
2017 , Volume 22, ¹ 6, p.35-47
Zhukov V.P., Bulgakova N.M., Fedoruk M.P.
The modelling of nonreciprocal writing
Volumetric modification of transparent materials by femtosecond laser pulses (FLP) is usually carried out in multipulse irradiation regimes by focusing of laser beam into material bulk. Theoretical investigations of multipulse regimes are usually limited to estimations which do not take into account laser light scattering by free electron plasma. This plasma is generated by ionization of both valence electrons and defects accumulated in the irradiation region from pulse to pulse and resulting in local changes of material refractive index. In this work, numerical modelling of FLP action on fused silica has been performed for multipulsed regime using focusing to the sample depth. The model is based on solution of non-linear Maxwell’s equations supplemented by the hydrodynamic-type equations for the plasma of electrons, which are excited by radiation to the conduction band. It takes into account effects connected with pulseto-pulse defect accumulation in glass. It is shown that accumulation of defects (color centers in glass), their ionization by subsequent laser pulses, and refractive index variation connected with color centers play a crucial role in the dynamics of radiation absorption in the multipulse regimes of glass modification. Additionally, in a number of experiments on multipulse writing of modification structures to the bulk of moving material samples, we observe the dependence of modification degree on the direction of sample motion relative to the laser beam (writing anisotropy). The effect of such asymmetric writing is usually explained by the tilted front of ultrashort laser beams. In the present work the numerical modelling of the action of the pulses with tilted front has been carried out for the first time and indeed it is shown that the tilted front could cause writing anisotropy.
[full text] Keywords: femtosecond laser pulses, defects, color centers, glass memory, multipulse regime, anisotropic writing, femtowriting, pulse front tilt, nonlinear Maxwells equations
Author(s): Zhukov Vladimir Petrovich Dr. Position: Senior Research Scientist Office: Federal Research Center for Information and Computational Technologies Address: 630090, Russia, Novosibirsk, Ac. Lavrentiev ave., 6
Phone Office: (383) 330 97 72 E-mail: zuk@ict.nsc.ru Bulgakova Nadezhda Mikhailovna Dr. , Senior Scientist Position: General Scientist Office: Kutateladze Institute of Thermophysics Siberian Branch of the RAS Address: 630090, Russia, Novosibirsk, 1, Ac. Lavrentieva ave
Phone Office: (383) 330-70-50 E-mail: nbul@itp.nsc.ru Fedoruk Mikhail Petrovich Dr. , Academician RAS, Professor Position: Chancellor Office: Novosibirsk State University, Federal Research Center for Information and Computational Technologies Address: 630090, Russia, Novosibirsk, str. Pirogova, 2
Phone Office: (3832) 349105 E-mail: mife@net.ict.nsc.ru SPIN-code: 4929-8753 References: [1] Dostovalov, A.V., Babin, S.A., Wolf, A.A., Dubov, M.V., Mezentsev, V.K. Numerical investigation of the effect of the temporal pulse shape on modification of fused silica by femtosecond pulses. Quantum Electronics. 2012; 42(9):799-804. [2] Zhukov, V.P., Rubenchik, A.M., Fedoruk, M.P., Bulgakova, N.M. Interaction of doughnut-shaped laser pulses with glasses. JOSA B. 2017; 34(2):463–471. [3] Akturk, S., Gu, X., Gabolde, P., Trebino, R. The general theory of first-order spatiotemporal distortion of Gaussian pulses and beams. Optic Express. 2005; 13(21):8642–8661. [4] Kammel, R., Ackerman, R., Thomas, J., Skupin, S., Turnnermann, A., Nolte, S. Enhancing precision in fs-laser material processing by simultaneous spatial and temporal focusing. Light: Science and Applications. 2014; (3): e169. DOI:10.1038/lsa.2014.50. [5] Vitek, D.N., Block, E., Bellouard, Y., Adams, D.E., Backus, S., Kleinfeld, D., Durfee, Ch.G., Squier, J.A. Spatio-temporally focused femtosecond laser pulses for nonreciprocal writing in optically transparent materials. Optics Express. 2010; 18(24):24673-24678. [6] Kazansky, P.G., Yang, W., Bricchi, E., Bovatsek, J., Arai, A. et al. “Quill” writing with ultrashort light pulses in transparent materials. Applied Physics Letters.2007; 90(15):151120. [7] Kazansky, P.G., Shimotsuma, Y., Sakakura, M., Beresna, M., Gecevicius, M., Svirko, Y., Akturk, S., Qiu, J., Miura, K., Hirao, K. Photosensitivity control of an isotropic medium through polarization of light pulses with tilted intensity front. Optics Express. 2011; 19(21):20657–20664. [8] Bulgakova, N.M., Zhukov, V.P. Continuum models of ultrashort laser - matter interaction in application to wide-bandgap dielectrics. Springer Series in Materials Science. Laser in Materials Science. Eds. M. Castillejo, P.M. Ossi, L. Zhigilei. 2014; (191):101–124. [9] Bulgakova, N.M., Zhukov, V.P., Meshcheryakov, Yu.P. Theoretical treatments of ultrashort pulse laser processing of transparent materials: Towards understanding the volume nanograting formation and “quill” writing effect. Applied Physics B. 2013; 113(3):437– 449. [10] Bulgakova, N.M., Zhukov, V.P., Meshcheryakov, Yu.P., Gemini, L., Brajer, J., Rostohar, D., Mocek, T. Pulsed laser modification of transparent dielectrics: What can be foreseen and predicted in numerical experiments. Journal of the Optical Society of America. B. 2014; 31(11):C8–C14. [11] Bulgakova, N.M., Zhukov, V.P., Sonina, S.V., Meshcheryakov, Yu.P. Modification of transparent materials with ultrashort laser pulses: What is energetically and mechanically meaningful? Journal of Applied Physics. 2015; 118(23): Paper 233108 (17 p.) [12] Couairon, A., Sudrie, L., Franco, M., Pride, B., Mysyrowicz, A. Filamintation and damage in fused silica induced by tightly focused femtosecond laser pulses. Physical Review B. 2005; (71):125435 (11 p.) [13] Zhukov, V.P., Bulgakova, N.M., Fedoruk M.P. Numerical modeling of propagation of femtosecond laser pulses in non-linear media. Computational Technologies. 2012; 17(4):14–28. (In Russ.) [14] Martin, P., Guizard, S., Daguzan, Ph., Petite, G., D’Oliveira, P., Maynadier, P., Pedrix, M. Subpicosecond study of carrier trapping dynamics in wide-band-gap crystals. Physical Review B. 1997; (55):5799–5810. [15] Hecht, B., Novotny, L. Principles of Nano-Optics. Chapter 3: Propagation and focusing of optical fields. Cambridge University Press; 2006:578. [16] Grojo, D., Gertsvolf, M., Lei, S., Barillot, T., Rayner, D.M., Corkum, P.B. Excitonseeded multiphoton ionization in bulk SiO2. Physical Review B. 2010; (81):212301 (4 p.) [17] Petite, G., Guizard, S., Martin, P., Qu´er´e, F. Comment on “Ultrafast electron dynamics in femtosecond optical breakdown of dielectrics”. Physical Review B. 1999; (83):5182.
Bibliography link: Zhukov V.P., Bulgakova N.M., Fedoruk M.P. The modelling of nonreciprocal writing // Computational technologies. 2017. V. 22. ¹ 6. P. 35-47
|